Lab logoShuai Zhang Group @ ZJU
Graphene interface background

Research

Current Research

Research at the Shuai Zhang Group focuses on interfacial mechanics and its intersections with materials science, chemistry, and condensed matter physics. We seek to uncover the fundamental principles governing interfaces and use these insights to understand, design, and tune the mechanical, electrical, and physical properties of materials.

Tribology at Nanoscale

Controlling, and in many cases minimizing, friction is a goal that has long been pursued in history. From the classic Amontons–Coulomb law to the recent nanoscale experiments, the steady-state friction is found to be an inherent property of a sliding interface, which typically cannot be altered on demand. Two-dimensional materials, with atomically flat surfaces and highly tunable structures, offer a unique platform for understanding the microscopic origins of friction and dynamically regulating interfacial friction.

Thickness-dependent friction on CuInP₂S₆

Unusual Thickness-Dependent Friction on CuInP2S6 Originating from Work-Function Regulation

An unusual thickness-dependent friction was observed on ferroelectric CuInP2S6, opposite to the conventional trend. We attribute this to thickness-dependent work function and charge transfer. This work sheds light on the physical origins of friction for ferroelectric materials and suggests an effective strategy to actively regulate friction via work-function engineering.

See also: Chen, Z., et al., Unusual Thickness-Dependent Friction on CuInP2S6 Originating from Work-Function Regulation, Physical Review Letters (2025)

Dual-scale stick-slip friction map

Dual-Scale Stick-Slip Friction on Graphene/h-BN Moiré Superlattice Structure

We observed unique dual-scale stick–slip on graphene/h-BN. We attribute the moiré-scale behavior to the accumulation and sudden release of strain in graphene. These results highlight the strong influence of interfacial states on the dynamics and energy dissipation of 2D structures.

See also: Zhang, S., et al., Dual-Scale Stick-Slip Friction on Graphene/h-BN Moiré Superlattice Structure, Physical Review Letters (2022)

In the news: Tsinghua News

Mechanics of Twisted Interfaces

Twisting van der Waals interfaces provides a powerful means to regulate interlayer coupling and engineer the physical properties of two-dimensional materials. We explore the rich mechanical phenomena emerging at these buried interfaces and harness them to understand and manipulate structural, electronic, and other emergent behaviors in twisted materials.

Conductive AFM of a twisted multilayer interface

Deducing the Internal Interfaces of Twisted Multilayer Graphene via Moiré-Regulated Surface Conductivity

We developed a conductive AFM-based method for characterizing buried interfaces in twisted van der Waals structures. By establishing a correlation between surface conductivity and internal stacking configurations, this approach enables the reconstruction of buried interfacial structures from simple conductivity mapping.

See also: Wang, H., et al., Deducing the internal interfaces of twisted multilayer graphene via moiré-regulated surface conductivity, National Science Review (2023)

In the news: National Science Review and Tsinghua News

Domino-like stacking order switching

Domino-like Stacking Order Switching in Twisted Monolayer–Multilayer Graphene

Two metastable reconstruction states with distinct stacking orders were observed in small-angle twisted monolayer–multilayer graphene. These states can be reversibly switched through a domino-like propagation process driven by strong mechanical coupling among solitons, providing a new route to manipulate stacking configurations in twisted van der Waals structures.

See also: Zhang, S., et al., Domino-like stacking order switching in twisted monolayer–multilayer graphene, Nature Materials (2022)

In the news: Nature Materials News & Views and Tsinghua News

Conductivity map in low-angle twisted bilayer graphene

Abnormal Conductivity in Low-Angle Twisted Bilayer Graphene

We report a nonmonotonic angle-dependent vertical conductivity across the interface of bilayer graphene with low twist angles. The abnormal behavior is attributed to the unusual reduction in average carrier density originating from local atomic reconstruction. These results highlight the key role of atomic reconstruction in tuning electronic transport in twisted van der Waals materials.

See also: Zhang, S., et al., Abnormal conductivity in low-angle twisted bilayer graphene, Science Advances (2020)

In the news: Phys.org News and Tsinghua News

Mechanochemistry

Mechanochemistry explores how mechanical forces drive chemical reactions and material transformations. We seek to uncover how stress and strain reshape reaction pathways and energy landscapes at interfaces, and harness these effects to create new materials and engineer novel devices beyond the reach of conventional thermal processes.